In the Sky Protect app, you can add or uninstall devices (Chime, video doorbell, contact sensors, motion sensors and leak sensors) by selecting Devices under Settings.
You can only change a device as above as a Primary user.
If you have created a secondary user for another member of your household, they cannot change devices.
If by device you mean you have changed to a different phone/tablet, just login to the Sky Protect app with your Sky email and password you currently use on your phone/tablet device and login. You do not need to remove the older phone/tablet, just log out of the Sky Protect app on it and login with either the Primary or Secondary email and password you were previously using.
You can run as a Primary user on multiole phones and tablets at the same time, if you so wish..
A secondary user can do everything a primary user can except remove and add other users/devices (Chime, video doorbell, contact sensors, motion sensors and leak sensors) or change consent settings
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